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Facile surfactant-assisted synthesis of CTAB-incorporated MoS2 ultrathin nanosheets for efficient hydrogen evolution

  • 发布时间:2021-03-15
  • 点击次数:

  • 关键字:HYDROTHERMAL SYNTHESIS; WS2 NANOSHEETS; ELECTROCATALYST; CATALYST; NANOPARTICLES; PERFORMANCE; GRAPHENE; EXFOLIATION; HYBRIDS
  • 摘要:Molybdenum disulfide (MoS2) has emerged as a promising electrocatalyst for catalyzing protons to hydrogen via the so-called hydrogen evolution reaction (HER). In order to enhance the HER activity, CTAB (cetyltrimethyl ammonium bromide)-incorporated MoS2 ultrathin nanosheets with high specific surface area and more catalytic active sites have been successfully synthesized via a facile surfactant-assisted hydrothermal approach. Adding CTAB to the hydrothermal process can effectively regulate both structural and electronic benefits by controllable disorder engineering and simultaneous CTAB incorporation in MoS2 catalysts, leading to a higher specific surface area, more catalytic active sites and better electrical conductivity for improving HER activity. The optimized CTAB-incorporated MoS2 ultrathin nanosheets exhibit excellent activity for HER with a small onset potential of 88 mV, a low Tafel slope of 55 mV dec(-1), and relatively good stability.
  • 卷号:6
  • 期号:20
  • 是否译文:

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