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Bioinspired, High-Strength, and Flexible MXene/Aramid Fiber for Electromagnetic Interference Shielding Papers with Joule Heating Performance

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Key Words:CARBON NANOFIBER; COMPOSITE FOAMS; MECHANICAL-PROPERTIES; MXENE FILMS; LIGHTWEIGHT; ABSORPTION; ULTRATHIN; SURFACE; NANOCOMPOSITES; CELLULOSE

Abstract:High-strength, flexible, and multifunctional characteristics are highly desirable for electromagnetic interference (EMI) shielding materials in the field of electric devices. In this work, inspired by natural nacre, we fabricated large-scale, layered MXene/amarid nanofiber (ANF) nanocomposite papers by blade-coating process plus sol-gel conversion step. The as-synthesized papers possess excellent mechanical performance, that is, exceptional tensile strength (198.80 +/- 5.35 MPa), large strain (15.30 +/- 1.01%), and good flexibility (folded into various models without fracture), which are ascribed to synergetic interactions of the interconnected three-dimensional network frame and hydrogen bonds between MXene and ANF. More importantly, the papers with extensive continuous conductive paths formed by MXene nanosheets present a high EMI shielding effectiveness of 13188.2 dB cm(2) g(-1) in the frequency range of 8.2-12.4 GHz. More interestingly, the papers show excellent Joule heating performance with a fast thermal response (<10 s) and a low driving voltage (<= 4 V). As such, the large-scale MXene/ANF papers are considered as promising alternatives in a wide range of applications in electromagnetic shielding and thermal management.

Volume:16

Issue:4

Translation or Not:no