青岛科技大学  English 
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教授 博士生导师  
硕士生导师  

教师拼音名称:linjianjian

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入职时间:2018-09-11

所在单位:化学与分子工程学院

学历:博士研究生

办公地点:四方校区第一实验楼216

性别:女

联系方式:19862229511

学位:工学博士

职称:教授

毕业院校:澳大利亚伍伦贡大学

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Durable Broadband and Omnidirectional Ultra-antireflective Surfaces

关键字:Fused silica;Antireflection coatings - Coatings - Display devices - Durability - Energy conversion - Lenses - Light reflection - Monolayers - Optoelectronic devices - Solar energy - Sols

摘要:Light reflection from surfaces is ubiquitous in nature. Diverse optoelectronic devices need durable, omnidirectional, and transparent ultra-antireflective surfaces. Here, we engineered antireflective transparent surfaces composed of silica nanocaps through a simple thermal treatment of a silica-coated monolayer colloidal crystal template. The relationship between the structure and the antireflective performance of the silica nanocaps was systematically studied both experimentally and numerically. On the basis of the understanding of the structure-antireflection relationships, ultra-antireflection coatings with a transmittance of ∼98.75 ± 0.15% in the visible wavelength range were prepared by fabricating two differently sized silica nanocaps. More importantly, the antireflection of the coatings formed by two differently sized nanocaps demonstrated poor dependence on the angle of the incident light (i.e., omnidirectionality). The reflection is <2.5% even at an incident angle of 60°. The prepared ultra-antireflective silica nanocap coatings outperform state-of-the-art transparent antireflective coatings regarding the antireflection performance, the wavelength range, and the omnidirectionality. The silica nanoshells were welded together with the underlying fused silica. Therefore, they can sustain common mechanical friction and scratching, demonstrating extraordinary mechanical durability as verified by sand abrasion tests. Further, the silanized silica nanocaps turned out to be hydrophobic with an outstanding self-cleaning performance without prominently influencing the transmittance. The durable and omnidirectional ultra-antireflective transparent silica nanocaps will have promising applications in solar energy conversion and storage, displays, optical lenses, and a wide range of optoelectronic devices.<br/> Copyright © 2018 American Chemical Society.

卷号:10

期号:46

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